All Publications


  • Local probe of bulk and edge states in a fractional Chern insulator. Nature Ji, Z., Park, H., Barber, M. E., Hu, C., Watanabe, K., Taniguchi, T., Chu, J. H., Xu, X., Shen, Z. X. 2024; 635 (8039): 578-583

    Abstract

    The fractional quantum Hall effect is a key example of topological quantum many-body phenomena, arising from the interplay between strong electron correlation, topological order and time-reversal symmetry breaking. Recently, a lattice analogue of the fractional quantum Hall effect at zero magnetic field has been observed, confirming the existence of a zero-field fractional Chern insulator (FCI). Despite this, the bulk-edge correspondence-a hallmark of a FCI featuring an insulating bulk with conductive edges-has not been directly observed. In fact, this correspondence has not been visualized in any system for fractional states owing to experimental challenges. Here we report the imaging of FCI edge states in twisted MoTe2 (t-MoTe2) using microwave impedance microscopy1. By tuning the carrier density, we observe the system evolving between metallic and FCI states, the latter of which exhibits insulating bulk and conductive edges, as expected from the bulk-boundary correspondence. Further analysis suggests the composite nature of the FCI edge states. We also observe the evolution of edge states across the topological phase transition as a function of interlayer electric field and reveal exciting prospects of neighbouring domains with different fractional orders. These findings pave the way for research into topologically protected one-dimensional interfaces between various anyonic states at zero magnetic field, such as gapped one-dimensional symmetry-protected phases with non-zero topological entanglement entropy, Halperin-Laughlin interfaces and the creation of non-abelian anyons.

    View details for DOI 10.1038/s41586-024-08092-7

    View details for PubMedID 39567787

    View details for PubMedCentralID 11464376

  • Opto-twistronic Hall effect in a three-dimensional spiral lattice. Nature Ji, Z., Zhao, Y., Chen, Y., Zhu, Z., Wang, Y., Liu, W., Modi, G., Mele, E. J., Jin, S., Agarwal, R. 2024

    Abstract

    Studies of moiré systems have explained the effect of superlattice modulations on their properties, demonstrating new correlated phases1. However, most experimental studies have focused on a few layers in two-dimensional systems. Extending twistronics to three dimensions, in which the twist extends into the third dimension, remains underexplored because of the challenges associated with the manual stacking of layers. Here we study three-dimensional twistronics using a self-assembled twisted spiral superlattice of multilayered WS2. Our findings show an opto-twistronic Hall effect driven by structural chirality and coherence length, modulated by the moiré potential of the spiral superlattice. This is an experimental manifestation of the noncommutative geometry of the system. We observe enhanced light-matter interactions and an altered dependence of the Hall coefficient on photon momentum. Our model suggests contributions from higher-order quantum geometric quantities to this observation, providing opportunities for designing quantum-materials-based optoelectronic lattices with large nonlinearities.

    View details for DOI 10.1038/s41586-024-07949-1

    View details for PubMedID 39294380

    View details for PubMedCentralID 10439888

  • Characterization of Two Fast-Turnaround Dry Dilution Refrigerators for Scanning Probe Microscopy JOURNAL OF LOW TEMPERATURE PHYSICS Barber, M. E., Li, Y., Gibson, J., Yu, J., Jiang, Z., Hu, Y., Ji, Z., Nandi, N., Hoke, J. C., Bishop-Van Horn, L., Arias, G. R., Van Harlingen, D. J., Moler, K. A., Shen, Z., Kou, A., Feldman, B. E. 2024
  • Capturing dynamical correlations using implicit neural representations. Nature communications Chitturi, S. R., Ji, Z., Petsch, A. N., Peng, C., Chen, Z., Plumley, R., Dunne, M., Mardanya, S., Chowdhury, S., Chen, H., Bansil, A., Feiguin, A., Kolesnikov, A. I., Prabhakaran, D., Hayden, S. M., Ratner, D., Jia, C., Nashed, Y., Turner, J. J. 2023; 14 (1): 5852

    Abstract

    Understanding the nature and origin of collective excitations in materials is of fundamental importance for unraveling the underlying physics of a many-body system. Excitation spectra are usually obtained by measuring the dynamical structure factor, S(Q, ω), using inelastic neutron or x-ray scattering techniques and are analyzed by comparing the experimental results against calculated predictions. We introduce a data-driven analysis tool which leverages 'neural implicit representations' that are specifically tailored for handling spectrographic measurements and are able to efficiently obtain unknown parameters from experimental data via automatic differentiation. In this work, we employ linear spin wave theory simulations to train a machine learning platform, enabling precise exchange parameter extraction from inelastic neutron scattering data on the square-lattice spin-1 antiferromagnet La2NiO4, showcasing a viable pathway towards automatic refinement of advanced models for ordered magnetic systems.

    View details for DOI 10.1038/s41467-023-41378-4

    View details for PubMedID 37730824

    View details for PubMedCentralID 8662964

  • Generation of helical topological exciton-polaritons SCIENCE Liu, W., Ji, Z., Wang, Y., Modi, G., Hwang, M., Zheng, B., Sorger, V. J., Pan, A., Agarwal, R. 2020; 370 (6516): 600-604

    Abstract

    Topological photonics in strongly coupled light-matter systems offer the possibility for fabricating tunable optical devices that are robust against disorder and defects. Topological polaritons, i.e., hybrid exciton-photon quasiparticles, have been proposed to demonstrate scatter-free chiral propagation, but their experimental realization to date has been at deep cryogenic temperatures and under strong magnetic fields. We demonstrate helical topological polaritons up to 200 kelvin without external magnetic field in monolayer WS2 excitons coupled to a nontrivial photonic crystal protected by pseudo time-reversal symmetry. The helical nature of the topological polaritons, where polaritons with opposite helicities are transported to opposite directions, is verified. Topological helical polaritons provide a platform for developing robust and tunable polaritonic spintronic devices for classical and quantum information-processing applications.

    View details for DOI 10.1126/science.abc4975

    View details for Web of Science ID 000583031800051

    View details for PubMedID 33033158

  • Tunable geometric photocurrent in van der Waals heterostructure OPTICA Rasmita, A., Jiang, C., Ma, H., Ji, Z., Agarwal, R., Gao, W. 2020; 7 (9): 1204-1208
  • Photocurrent detection of the orbital angular momentum of light SCIENCE Ji, Z., Liu, W., Krylyuk, S., Fan, X., Zhang, Z., Pan, A., Feng, L., Davydov, A., Agarwal, R. 2020; 368 (6492): 763-+

    Abstract

    Applications that use the orbital angular momentum (OAM) of light show promise for increasing the bandwidth of optical communication networks. However, direct photocurrent detection of different OAM modes has not yet been demonstrated. Most studies of current responses to electromagnetic fields have focused on optical intensity-related effects, but phase information has been lost. In this study, we designed a photodetector based on tungsten ditelluride (WTe2) with carefully fabricated electrode geometries to facilitate direct characterization of the topological charge of OAM of light. This orbital photogalvanic effect, driven by the helical phase gradient, is distinguished by a current winding around the optical beam axis with a magnitude proportional to its quantized OAM mode number. Our study provides a route to develop on-chip detection of optical OAM modes, which can enable the development of next-generation photonic circuits.

    View details for DOI 10.1126/science.aba9192

    View details for Web of Science ID 000535608300045

    View details for PubMedID 32409474

    View details for PubMedCentralID PMC7545405

  • Spatially dispersive circular photogalvanic effect in a Weyl semimetal NATURE MATERIALS Ji, Z., Liu, G., Addison, Z., Liu, W., Yu, P., Gao, H., Liu, Z., Rappe, A. M., Kane, C. L., Mele, E. J., Agarwal, R. 2019; 18 (9): 955-+

    Abstract

    Weyl semimetals (WSMs) are gapless topological states of matter with broken inversion and/or time reversal symmetry. WSMs can support a circulating photocurrent when illuminated by circularly polarized light at normal incidence. Here, we report a spatially dispersive circular photogalvanic effect (s-CPGE) in a WSM that occurs with a spatially varying beam profile. Our analysis shows that the s-CPGE is controlled by a symmetry selection rule combined with asymmetric carrier excitation and relaxation dynamics. By evaluating the s-CPGE for a minimal model of a WSM, a frequency-dependent scaling behaviour of the photocurrent is obtained. Wavelength-dependent measurements from the visible to mid-infrared range show evidence of Berry curvature singularities and band inversion in the s-CPGE response. We present the s-CPGE as a promising spectroscopic probe for topological band properties, with the potential for controlling photoresponse by patterning optical fields on topological materials to store, manipulate and transmit information.

    View details for DOI 10.1038/s41563-019-0421-5

    View details for Web of Science ID 000482186000015

    View details for PubMedID 31308515