Brian Kaufman
Research Assoc-Experimental, SLAC National Accelerator Laboratory
All Publications
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Long-lived electronic coherences in molecular wave packets probed with pulse-shape spectroscopy
PHYSICAL REVIEW A
2024; 110 (3)
View details for DOI 10.1103/PhysRevA.110.033118
View details for Web of Science ID 001327395600001
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Direct observation of entangled electronic-nuclear wave packets
PHYSICAL REVIEW RESEARCH
2024; 6 (2)
View details for DOI 10.1103/PhysRevResearch.6.L022047
View details for Web of Science ID 001239824300005
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High repetition-rate pulse shaping of a spectrally broadened Yb femtosecond laser
OPTICS CONTINUUM
2024; 3 (5): 785-794
View details for DOI 10.1364/OPTCON.522036
View details for Web of Science ID 001299663200006
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Long-Lived Electronic Coherences in Molecules
PHYSICAL REVIEW LETTERS
2023; 131 (26): 263202
Abstract
We demonstrate long-lived electronic coherences in molecules using a combination of measurements with shaped octave spanning ultrafast laser pulses and calculations of the light matter interaction. Our pump-probe measurements prepare and interrogate entangled nuclear-electronic wave packets whose electronic phase remains well defined despite vibrational motion along many degrees of freedom. The experiments and calculations illustrate how coherences between excited states can survive, even when coherence with the ground state is lost, and may have important implications for many areas of attosecond science and photochemistry.
View details for DOI 10.1103/PhysRevLett.131.263202
View details for Web of Science ID 001153471200005
View details for PubMedID 38215370
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Numerical calculations of multiphoton molecular absorption
PHYSICAL REVIEW A
2022; 106 (1)
View details for DOI 10.1103/PhysRevA.106.013111
View details for Web of Science ID 000835592900007
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A simple approach for characterizing the spatially varying sensitivity of microchannel plate detectors
REVIEW OF SCIENTIFIC INSTRUMENTS
2022; 93 (7): 075108
Abstract
We present a simple approach to characterize the spatial variation of the gain in microchannel plate (MCP) coupled to phosphor detectors using single electron or photon hits. The technique is easy to implement and general enough to be extended to other kinds of detectors. We demonstrate the efficacy of the approach on both laboratory and Monte Carlo generated datasets. Furthermore, we use the approach to measure the variation in gain over time as the MCP is exposed to an increasing number of electrons.
View details for DOI 10.1063/5.0092346
View details for Web of Science ID 000936216500008
View details for PubMedID 35922295
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Acousto-optic modulator pulse-shaper compression of octave-spanning pulses from a stretched hollow-core fiber
OSA CONTINUUM
2021; 4 (12): 3176-3183
View details for DOI 10.1364/OSAC.440476
View details for Web of Science ID 000732743000007
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Competition between dynamic resonance and internal conversion in strong-field molecular ionization with chirped ultrafast laser pulses
PHYSICAL REVIEW A
2021; 103 (2)
View details for DOI 10.1103/PhysRevA.103.023108
View details for Web of Science ID 000618066800009
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Adiabatic elimination in strong-field light-matter coupling
PHYSICAL REVIEW A
2020; 102 (6)
View details for DOI 10.1103/PhysRevA.102.063117
View details for Web of Science ID 000601327400008
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Coherent Control of Internal Conversion in Strong-Field Molecular Ionization
PHYSICAL REVIEW LETTERS
2020; 125 (5): 053202
Abstract
We demonstrate coherent control over internal conversion during strong-field molecular ionization with shaped, few-cycle laser pulses. The control is driven by interference in different neutral states, which are coupled via non-Born-Oppenheimer terms in the molecular Hamiltonian. Our measurements highlight the preservation of electronic coherence in nonadiabatic transitions between electronic states.
View details for DOI 10.1103/PhysRevLett.125.053202
View details for Web of Science ID 000553250400008
View details for PubMedID 32794883
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Time-resolved measurement of internal conversion dynamics in strong-field molecular ionization
PHYSICAL REVIEW A
2017; 96 (2)
View details for DOI 10.1103/PhysRevA.96.021401
View details for Web of Science ID 000406749100001