All Publications


  • Terahertz Radiation of Plasmonic Hot Carriers Taghinejad, M., Xia, C., Hrton, M., Lee, K., Kim, A. S., Li, Q., Guzelturk, B., Kalousek, R., Xu, F., Cai, W., Lindenberg, A. M., Brongersma, M. L., Lin, S. Y., Adibi, A., Scherer, A. SPIE-INT SOC OPTICAL ENGINEERING. 2024

    View details for DOI 10.1117/12.3010182

    View details for Web of Science ID 001209319500001

  • Determining hot-carrier transport dynamics from terahertz emission. Science (New York, N.Y.) Taghinejad, M., Xia, C., Hrton, M., Lee, K. T., Kim, A. S., Li, Q., Guzelturk, B., Kalousek, R., Xu, F., Cai, W., Lindenberg, A. M., Brongersma, M. L. 2023; 382 (6668): 299-305

    Abstract

    Understanding the ultrafast excitation and transport dynamics of plasmon-driven hot carriers is critical to the development of optoelectronics, photochemistry, and solar-energy harvesting. However, the ultrashort time and length scales associated with the behavior of these highly out-of-equilibrium carriers have impaired experimental verification of ab initio quantum theories. Here, we present an approach to studying plasmonic hot-carrier dynamics that analyzes the temporal waveform of coherent terahertz bursts radiated by photo-ejected hot carriers from designer nano-antennas with a broken symmetry. For ballistic carriers ejected from gold antennas, we find an ~11-femtosecond timescale composed of the plasmon lifetime and ballistic transport time. Polarization- and phase-sensitive detection of terahertz fields further grant direct access to their ballistic transport trajectory. Our approach opens explorations of ultrafast carrier dynamics in optically excited nanostructures.

    View details for DOI 10.1126/science.adj5612

    View details for PubMedID 37856614

  • A Purcell-enabled monolayer semiconductor free-space optical modulator NATURE PHOTONICS Li, Q., Song, J., Xu, F., van de Groep, J., Hong, J., Daus, A., Lee, Y., Johnson, A. C., Pop, E., Liu, F., Brongersma, M. L. 2023
  • Quantitative phase contrast imaging with a nonlocal angle-selective metasurface. Nature communications Ji, A., Song, J. H., Li, Q., Xu, F., Tsai, C. T., Tiberio, R. C., Cui, B., Lalanne, P., Kik, P. G., Miller, D. A., Brongersma, M. L. 2022; 13 (1): 7848

    Abstract

    Phase contrast microscopy has played a central role in the development of modern biology, geology, and nanotechnology. It can visualize the structure of translucent objects that remains hidden in regular optical microscopes. The optical layout of a phase contrast microscope is based on a 4 f image processing setup and has essentially remained unchanged since its invention by Zernike in the early 1930s. Here, we propose a conceptually new approach to phase contrast imaging that harnesses the non-local optical response of a guided-mode-resonator metasurface. We highlight its benefits and demonstrate the imaging of various phase objects, including biological cells, polymeric nanostructures, and transparent metasurfaces. Our results showcase that the addition of this non-local metasurface to a conventional microscope enables quantitative phase contrast imaging with a 0.02π phase accuracy. At a high level, this work adds to the growing body of research aimed at the use of metasurfaces for analog optical computing.

    View details for DOI 10.1038/s41467-022-34197-6

    View details for PubMedID 36543788

    View details for PubMedCentralID PMC9772391