Yigao Yuan
Postdoctoral Scholar, Materials Science and Engineering
Bio
heterogeneous photocatalysis
Professional Education
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Bachelor of Science, Nanjing University, Chemistry (2019)
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Master of Arts, Rice University (2021)
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Doctor of Philosophy, Rice University (2024)
All Publications
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Steam methane reforming using a regenerable antenna-reactor plasmonic photocatalyst
NATURE CATALYSIS
2024; 7 (12): 1339-1349
View details for DOI 10.1038/s41929-024-01248-8
View details for Web of Science ID 001345891800001
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Earth-abundant photocatalyst for H2 generation from NH3 with light-emitting diode illumination.
Science (New York, N.Y.)
2022; 378 (6622): 889-893
Abstract
Catalysts based on platinum group metals have been a major focus of the chemical industry for decades. We show that plasmonic photocatalysis can transform a thermally unreactive, earth-abundant transition metal into a catalytically active site under illumination. Fe active sites in a Cu-Fe antenna-reactor complex achieve efficiencies very similar to Ru for the photocatalytic decomposition of ammonia under ultrafast pulsed illumination. When illuminated with light-emitting diodes rather than lasers, the photocatalytic efficiencies remain comparable, even when the scale of reaction increases by nearly three orders of magnitude. This result demonstrates the potential for highly efficient, electrically driven production of hydrogen from an ammonia carrier with earth-abundant transition metals.
View details for DOI 10.1126/science.abn5636
View details for PubMedID 36423268
https://orcid.org/0000-0003-1385-2395