Dr. Christopher T. Parzyck
Postdoctoral Scholar, Photon Science, SLAC
Bio
My research interests lie at the intersection of materials science and condensed matter physics. I work on thin film synthesis of oxide and metal systems by molecular-beam epitaxy (MBE). Applications range from answering fundamental physics questions about high temperature superconductivity to developing practical synthesis routines and new materials for next generation electron sources. In addition, I work on projects involving spectroscopic probes of thin film systems, including angle-resolved photoemission spectroscopy (ARPES) and resonant soft x-ray scattering (RSXS) measurements.
Professional Education
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Doctor of Philosophy, Cornell University, Physics (2023)
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Master of Science, Cornell University, Physics (2019)
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Master of Science, The University of New Mexico, Mathematics (2016)
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Bachelor of Science, University of California, San Diego, Physics & Mathematics (2013)
All Publications
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Is Ba<sub>3</sub>In<sub>2</sub>O<sub>6</sub> a high-<i>T<sub>c</sub> </i> superconductor?
JOURNAL OF PHYSICS-CONDENSED MATTER
2024; 36 (31)
Abstract
It has been suggested that Ba3In2O6might be a high-Tcsuperconductor. Experimental investigation of the properties of Ba3In2O6was long inhibited by its instability in air. Recently epitaxial Ba3In2O6with a protective capping layer was demonstrated, which finally allows its electronic characterization. The optical bandgap of Ba3In2O6is determined to be 2.99 eV in-the (001) plane and 2.83 eV along thec-axis direction by spectroscopic ellipsometry. First-principles calculations were carried out, yielding a result in good agreement with the experimental value. Various dopants were explored to induce (super-)conductivity in this otherwise insulating material. NeitherA- norB-site doping proved successful. The underlying reason is predominately the formation of oxygen interstitials as revealed by scanning transmission electron microscopy and first-principles calculations. Additional efforts to induce superconductivity were investigated, including surface alkali doping, optical pumping, and hydrogen reduction. To probe liquid-ion gating, Ba3In2O6was successfully grown epitaxially on an epitaxial SrRuO3bottom electrode. So far none of these efforts induced superconductivity in Ba3In2O6,leaving the answer to the initial question of whether Ba3In2O6is a high-Tcsuperconductor to be 'no' thus far.
View details for DOI 10.1088/1361-648X/ad42f3
View details for Web of Science ID 001219447200001
View details for PubMedID 38657622
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Surface reconstructions and electronic structure of metallic delafossite thin films
APL MATERIALS
2024; 12 (8)
View details for DOI 10.1063/5.0217540
View details for Web of Science ID 001291956900004
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Absence of 3<i>a</i><sub>0</sub> charge density wave order in the infinite-layer nickelate NdNiO<sub>2</sub>
NATURE MATERIALS
2024; 23 (4): 486-491
Abstract
A hallmark of many unconventional superconductors is the presence of many-body interactions that give rise to broken-symmetry states intertwined with superconductivity. Recent resonant soft X-ray scattering experiments report commensurate 3a0 charge density wave order in infinite-layer nickelates, which has important implications regarding the universal interplay between charge order and superconductivity in both cuprates and nickelates. Here we present X-ray scattering and spectroscopy measurements on a series of NdNiO2+x samples, which reveal that the signatures of charge density wave order are absent in fully reduced, single-phase NdNiO2. The 3a0 superlattice peak instead originates from a partially reduced impurity phase where excess apical oxygens form ordered rows with three-unit-cell periodicity. The absence of any observable charge density wave order in NdNiO2 highlights a crucial difference between the phase diagrams of cuprate and nickelate superconductors.
View details for DOI 10.1038/s41563-024-01797-0
View details for Web of Science ID 001152202500001
View details for PubMedID 38278983
View details for PubMedCentralID PMC10990928