
Yangfan Liu
Ph.D. Student in Earth System Science, admitted Autumn 2023
Education & Certifications
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Bachelor of Science, Nanjing University, Geochemistry (2023)
All Publications
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Aerosol light absorption alleviates particulate pollution during wintertime haze events.
Proceedings of the National Academy of Sciences of the United States of America
2025; 122 (1): e2402281121
Abstract
Aerosol light absorption has been widely considered as a contributing factor to the worsening of particulate pollution in large urban areas, primarily through its role in stabilizing the planetary boundary layer (PBL). Here, we report that absorption-dominated aerosol-radiation interaction can decrease near-surface fine particulate matter concentrations ([PM2.5]) at a large-scale during wintertime haze events. A "warm bubble" effect by the significant heating rate of absorbing aerosols above the PBL top generates a secondary circulation, enhancing the upward motion (downward motion) and the convergence (divergence) in polluted (relatively clean) areas, with a net effect of lowering near-surface [PM2.5]. Furthermore, aerosol absorption of ultraviolet-wave light effectively reduces the photolysis of chemical species, i.e., aerosol-photolysis interaction, hindering ozone formation, reducing atmospheric oxidizing capability, and suppressing secondary aerosol concentrations. Our model assessment reveals that the synergetic two effects decrease near-surface [PM2.5] by around 7.4%, so the presence of light-absorbing aerosols can considerably alleviate particulate pollution during wintertime haze events. Such negative feedbacks to the aerosol loading should be considered in weather/climate prediction and health assessment models.
View details for DOI 10.1073/pnas.2402281121
View details for PubMedID 39715431
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Short-Lived Air Pollutants and Climate Forcers Through the Lens of the COVID-19 Pandemic
REVIEWS OF GEOPHYSICS
2024; 62 (4)
View details for DOI 10.1029/2022RG000773
View details for Web of Science ID 001373363100001